It's not as easy as what size bar.
There are many variables, as Brian mentioned. Saw power, chain speed and the size of wood you're cutting are most important. Bar length comes into play, but not much.
If you have a 3 foot bar on an 066, the best cutting speed will depend on the size of the log. A 20 inch log, with this set up, will be cut fastest with full sequsence, a 40 inch log will cut fastest with a full skip. The exact point where it pays to switch one way or another is up to you and your cutting style.
Our three foot bar gets about 4 or 5 cuts on average before it's dull. Sharpening that long thing is the worst job, IMO, so I use the full skip.
The 24 inch bars get one or the other chain, and personally I like the full skip, in spite of lost cutting time. We don't cut firewood, just saw logs and delimbing, so the lost time is minimal. Full comp is a little smoother and faster at the 24" length, the skip is easier to sharpen.
As a side note we run bigger sprokets than most and mod the saws(more variables).
You need to do some timed cut comparisons and decide for yourself.